High-entropy compounds, where multiple elements occupy a single crystallographic site in a highly disordered manner, challenge conventional understandings of electronic structure based on periodicity and well-defined band dispersion. Here, we report a detailed nuclear magnetic resonance study of the high-entropy superconductor (RuRhPdIr)0.6Pt0.4Sb, revealing a spatially homogeneous electronic environment in the normal state, in stark contrast to its crystallographically disordered lattice. The superconducting state exhibits a small but solid Hebel-Slichter coherence peak followed by a significant decrease in the nuclear spin-lattice relaxation rate, providing compelling evidence for fully gapped s-wave pairing. Our findings not only deepen the understanding of superconductivity in highly disordered quantum materials but also open a new pathway for exploring novel superconducting states in entropy-stabilized systems.
Reference
Uniform electronic states and 𝑠-wave superconductivity in a strongly disordered high-entropy compound 𝑋0.6Pt0.4Sb (𝑋 = Ru, Rh, Pd, Ir) Journal Article
In: Physical Review B, vol. 112, pp. L020508, 2025.